Wow Ian - DD67000 that's quite some exhalted company the the 4331 can keep up with!
The DD66000 inspired me to convert my beloved Klipsch KG 5.5's to a 2.5way after I inspected the crossover schematic.
I would ideally completely restore the old ladies. Especially seeing as they are that good comparatively.
And no I've not ever heard not seen an all original 4331 or 4333.
I'm in two minds about my way forward with the cabinets. Finding the original mid horns and CD's seems like a long shot in Australia or for a reasonable price anywhere these days. The crossovers even more unlikely.
I can mostly recreate and redesign the crossovers from original schematics and my own measurement rig.
I've toyed with using the modern JBL HL1425 with the D220ti as a near alternative tho not exact replacement to stay close to the original design and use the 2502's to again get close if not completely original.
I'd then use the 2445's with the 2226's to create a copy cinema series 4507 clone in a new enclosure.